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Creators/Authors contains: "Yi, Kan"

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  1. Abstract. Parameterizations that impact wet removal of black carbon (BC)remain uncertain in global climate models. In this study, we enhance thedefault wet deposition scheme for BC in the Community Earth System Model (CESM)to (a) add relevant physical processes that were not resolved in thedefault model and (b) facilitate understanding of the relative importanceof various cloud processes on BC distributions. We find that the enhancedscheme greatly improves model performance against HIPPO observationsrelative to the default scheme. We find that convection scavenging, aerosolactivation, ice nucleation, evaporation of rain or snow, and below-cloudscavenging dominate wet deposition of BC. BC conversion rates for processesrelated to in-cloud water–ice conversion (i.e., riming, the Bergeronprocess, and evaporation of cloud water sedimentation) are relativelysmaller, but have large seasonal variations. We also conduct sensitivitysimulations that turn off each cloud process one at a time to quantify theinfluence of cloud processes on BC distributions and radiative forcing.Convective scavenging is found to have the largest impact onBC concentrations at mid-altitudes over the tropics and even globally. Inaddition, BC is sensitive to all cloud processes over the NorthernHemisphere at high latitudes. As for BC vertical distributions, convectivescavenging greatly influences BC fractions at different altitudes.Suppressing BC droplet activation in clouds mainly decreases the fraction ofcolumn BC below 5 km, whereas suppressing BC ice nucleation increases thatabove 10 km. During wintertime, the Bergeron process also significantlyincreases BC concentrations at lower altitudes over the Arctic. Oursimulation yields a global BC burden of 85 Gg; corresponding directradiative forcing (DRF) of BC estimated using the Parallel Offline RadiativeTransfer (PORT) is 0.13 W m−2, much lower than previous studies. Therange of DRF derived from sensitivity simulations is large, 0.09–0.33 W m−2,corresponding to BC burdens varying from 73 to 151 Gg. Due todifferences in BC vertical distributions among each sensitivity simulation,fractional changes in DRF (relative to the baseline simulation) are alwayshigher than fractional changes in BC burdens; this occurs because relocating BCin the vertical influences the radiative forcing per BC mass. Our resultshighlight the influences of cloud microphysical processes on BC concentrationsand radiative forcing. 
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